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Role of substrate in the surface diffusion and kinetic roughening of nanocrystallised nickel electrodeposits

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Role of substrate in the surface diffusion and kinetic roughening of nanocrystallised nickel electrodeposits

Auteurs : RBID : Pascal:09-0197434

Descripteurs français

Pascal (Inist)
- Diffusion superficielle, Rugosité, Nickel, Revêtement électrodéposé, Dépôt électrolytique, Mécanisme croissance, Couche mince, Réseau cubique, Texture, Cristallite, Nanomatériau, Propriété surface, Propriété transport, Microscopie force atomique, Cuivre, Or, Oxyde d'étain, Oxyde d'indium, Coefficient diffusion, Régime hors équilibre, Longueur diffusion, Etude théorique, Ni, Substrat or, Substrat InSnO, 8115P, 8110A, 8107.
Wicri :
- concept : Nickel, Cuivre, Or.

English descriptors

KwdEn :
- Atomic force microscopy, Copper, Crystallites, Cubic lattices, Diffusion coefficient, Electrodeposited coatings, Electrodeposition, Gold, Growth mechanism, Indium oxide, Nanostructured materials, Nickel, Non equilibrium conditions, Roughness, Scattering lengths, Surface diffusion, Surface properties, Texture, Theoretical study, Thin films, Tin oxide, Transport properties.

Abstract

The surface growth and roughening of nano-crystallised Ni electrodeposits prepared at the same conditions have been studied on Cu, Au and ITO substrates. The Ni films obtained are characterised by the same face-centred cubic structure with a texture affected by the substrate chemical nature. Practically, the same small-sized grains of 83 nm mean height depicting a statistical mono-mode feature grow on Cu. A three-modal feature corresponding to the biggest and compact crystallites of 335, 368 and 400 nm mean height is obtained with Au. Two typical modes, respectively, linked to isolated big crystallites of 343 nm mean height and large zones of small grains of 170 nm height, result from the ITO effect. The surface transport properties of Ni ad-atoms on each substrate have been studied from the theoretical approach including the film global roughness measured by AFM. It is shown that the ad-atom diffusion coefficients (D_s) ranged in the interval 10^-10-10^-9cm²s^-1 are greatly affected by the non-equilibrium conditions of the film formation. Cu and ITO, respectively, lead to A_s=11.92 and 14.30 nm, while the higher D_s value and diffusion length A_s=37.32 nm are obtained with Au substrate.

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Pascal:09-0197434

Le document en format XML

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<author><name sortKey="Nzoghe Mendome, L" uniqKey="Nzoghe Mendome L">L. Nzoghe-Mendome</name>
<affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Laboratoire de Microscopies & d'Etude de Nanostructures, EA. no. 3799, UFR Sciences, Université de Reims, B.P. 138, 21 rue Clément Ader</s1>
<s2>51685 Reims</s2>
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<placeName><region type="region" nuts="2">Champagne-Ardenne</region>
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<author><name sortKey="Aloufy, A" uniqKey="Aloufy A">A. Aloufy</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Alexandria University, New Advanced Materials & Nanotechnology Center, Faculty of Engineering, Textile & Materials Engineering Department</s1>
<s2>21544 Alexandria</s2>
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<author><name sortKey="Ebothe, J" uniqKey="Ebothe J">J. Ebothe</name>
<affiliation wicri:level="3"><inist:fA14 i1="01"><s1>Laboratoire de Microscopies & d'Etude de Nanostructures, EA. no. 3799, UFR Sciences, Université de Reims, B.P. 138, 21 rue Clément Ader</s1>
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<author><name sortKey="El Messiry, M" uniqKey="El Messiry M">M. El Messiry</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Alexandria University, New Advanced Materials & Nanotechnology Center, Faculty of Engineering, Textile & Materials Engineering Department</s1>
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<sZ>4 aut.</sZ>
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<author><name sortKey="Hui, D" uniqKey="Hui D">D. Hui</name>
<affiliation wicri:level="1"><inist:fA14 i1="03"><s1>University of New Orleans, Department of Mechanical Engineering</s1>
<s2>New Orleans, LA 70148</s2>
<s3>USA</s3>
<sZ>5 aut.</sZ>
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<country>États-Unis</country>
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<publicationStmt><idno type="inist">09-0197434</idno>
<date when="2009">2009</date>
<idno type="stanalyst">PASCAL 09-0197434 INIST</idno>
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<seriesStmt><idno type="ISSN">0022-0248</idno>
<title level="j" type="abbreviated">J. cryst. growth</title>
<title level="j" type="main">Journal of crystal growth</title>
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</fileDesc>
<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Atomic force microscopy</term>
<term>Copper</term>
<term>Crystallites</term>
<term>Cubic lattices</term>
<term>Diffusion coefficient</term>
<term>Electrodeposited coatings</term>
<term>Electrodeposition</term>
<term>Gold</term>
<term>Growth mechanism</term>
<term>Indium oxide</term>
<term>Nanostructured materials</term>
<term>Nickel</term>
<term>Non equilibrium conditions</term>
<term>Roughness</term>
<term>Scattering lengths</term>
<term>Surface diffusion</term>
<term>Surface properties</term>
<term>Texture</term>
<term>Theoretical study</term>
<term>Thin films</term>
<term>Tin oxide</term>
<term>Transport properties</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Diffusion superficielle</term>
<term>Rugosité</term>
<term>Nickel</term>
<term>Revêtement électrodéposé</term>
<term>Dépôt électrolytique</term>
<term>Mécanisme croissance</term>
<term>Couche mince</term>
<term>Réseau cubique</term>
<term>Texture</term>
<term>Cristallite</term>
<term>Nanomatériau</term>
<term>Propriété surface</term>
<term>Propriété transport</term>
<term>Microscopie force atomique</term>
<term>Cuivre</term>
<term>Or</term>
<term>Oxyde d'étain</term>
<term>Oxyde d'indium</term>
<term>Coefficient diffusion</term>
<term>Régime hors équilibre</term>
<term>Longueur diffusion</term>
<term>Etude théorique</term>
<term>Ni</term>
<term>Substrat or</term>
<term>Substrat InSnO</term>
<term>8115P</term>
<term>8110A</term>
<term>8107</term>
</keywords>
<keywords scheme="Wicri" type="concept" xml:lang="fr"><term>Nickel</term>
<term>Cuivre</term>
<term>Or</term>
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<front><div type="abstract" xml:lang="en">The surface growth and roughening of nano-crystallised Ni electrodeposits prepared at the same conditions have been studied on Cu, Au and ITO substrates. The Ni films obtained are characterised by the same face-centred cubic structure with a texture affected by the substrate chemical nature. Practically, the same small-sized grains of 83 nm mean height depicting a statistical mono-mode feature grow on Cu. A three-modal feature corresponding to the biggest and compact crystallites of 335, 368 and 400 nm mean height is obtained with Au. Two typical modes, respectively, linked to isolated big crystallites of 343 nm mean height and large zones of small grains of 170 nm height, result from the ITO effect. The surface transport properties of Ni ad-atoms on each substrate have been studied from the theoretical approach including the film global roughness measured by AFM. It is shown that the ad-atom diffusion coefficients (D<sub>s</sub>
) ranged in the interval 10<sup>-10</sup>
-10<sup>-9</sup>
cm<sup>2</sup>
s<sup>-1</sup>
 are greatly affected by the non-equilibrium conditions of the film formation. Cu and ITO, respectively, lead to A<sub>s</sub>
=11.92 and 14.30 nm, while the higher D<sub>s</sub>
 value and diffusion length A<sub>s</sub>
=37.32 nm are obtained with Au substrate.</div>
</front>
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<fA11 i1="02" i2="1"><s1>ALOUFY (A.)</s1>
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<fA14 i1="01"><s1>Laboratoire de Microscopies & d'Etude de Nanostructures, EA. no. 3799, UFR Sciences, Université de Reims, B.P. 138, 21 rue Clément Ader</s1>
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<s3>FRA</s3>
<sZ>1 aut.</sZ>
<sZ>3 aut.</sZ>
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<fA14 i1="02"><s1>Alexandria University, New Advanced Materials & Nanotechnology Center, Faculty of Engineering, Textile & Materials Engineering Department</s1>
<s2>21544 Alexandria</s2>
<s3>EGY</s3>
<sZ>2 aut.</sZ>
<sZ>4 aut.</sZ>
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<fA14 i1="03"><s1>University of New Orleans, Department of Mechanical Engineering</s1>
<s2>New Orleans, LA 70148</s2>
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<fC01 i1="01" l="ENG"><s0>The surface growth and roughening of nano-crystallised Ni electrodeposits prepared at the same conditions have been studied on Cu, Au and ITO substrates. The Ni films obtained are characterised by the same face-centred cubic structure with a texture affected by the substrate chemical nature. Practically, the same small-sized grains of 83 nm mean height depicting a statistical mono-mode feature grow on Cu. A three-modal feature corresponding to the biggest and compact crystallites of 335, 368 and 400 nm mean height is obtained with Au. Two typical modes, respectively, linked to isolated big crystallites of 343 nm mean height and large zones of small grains of 170 nm height, result from the ITO effect. The surface transport properties of Ni ad-atoms on each substrate have been studied from the theoretical approach including the film global roughness measured by AFM. It is shown that the ad-atom diffusion coefficients (D<sub>s</sub>
) ranged in the interval 10<sup>-10</sup>
-10<sup>-9</sup>
cm<sup>2</sup>
s<sup>-1</sup>
 are greatly affected by the non-equilibrium conditions of the film formation. Cu and ITO, respectively, lead to A<sub>s</sub>
=11.92 and 14.30 nm, while the higher D<sub>s</sub>
 value and diffusion length A<sub>s</sub>
=37.32 nm are obtained with Au substrate.</s0>
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<fC02 i1="03" i2="3"><s0>001B80A07Z</s0>
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<fC03 i1="01" i2="3" l="FRE"><s0>Diffusion superficielle</s0>
<s5>01</s5>
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<fC03 i1="01" i2="3" l="ENG"><s0>Surface diffusion</s0>
<s5>01</s5>
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<fC03 i1="02" i2="3" l="FRE"><s0>Rugosité</s0>
<s5>02</s5>
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<fC03 i1="02" i2="3" l="ENG"><s0>Roughness</s0>
<s5>02</s5>
</fC03>
<fC03 i1="03" i2="3" l="FRE"><s0>Nickel</s0>
<s2>NC</s2>
<s5>03</s5>
</fC03>
<fC03 i1="03" i2="3" l="ENG"><s0>Nickel</s0>
<s2>NC</s2>
<s5>03</s5>
</fC03>
<fC03 i1="04" i2="3" l="FRE"><s0>Revêtement électrodéposé</s0>
<s5>04</s5>
</fC03>
<fC03 i1="04" i2="3" l="ENG"><s0>Electrodeposited coatings</s0>
<s5>04</s5>
</fC03>
<fC03 i1="05" i2="3" l="FRE"><s0>Dépôt électrolytique</s0>
<s5>05</s5>
</fC03>
<fC03 i1="05" i2="3" l="ENG"><s0>Electrodeposition</s0>
<s5>05</s5>
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<fC03 i1="06" i2="X" l="FRE"><s0>Mécanisme croissance</s0>
<s5>06</s5>
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<fC03 i1="06" i2="X" l="ENG"><s0>Growth mechanism</s0>
<s5>06</s5>
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<s5>06</s5>
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<s5>07</s5>
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<s5>07</s5>
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<s5>08</s5>
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<s5>08</s5>
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<s5>09</s5>
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<fC03 i1="09" i2="3" l="ENG"><s0>Texture</s0>
<s5>09</s5>
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<s5>10</s5>
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<s5>11</s5>
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<fC03 i1="12" i2="3" l="FRE"><s0>Propriété surface</s0>
<s5>12</s5>
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<fC03 i1="12" i2="3" l="ENG"><s0>Surface properties</s0>
<s5>12</s5>
</fC03>
<fC03 i1="13" i2="X" l="FRE"><s0>Propriété transport</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="ENG"><s0>Transport properties</s0>
<s5>13</s5>
</fC03>
<fC03 i1="13" i2="X" l="SPA"><s0>Propiedad transporte</s0>
<s5>13</s5>
</fC03>
<fC03 i1="14" i2="3" l="FRE"><s0>Microscopie force atomique</s0>
<s5>14</s5>
</fC03>
<fC03 i1="14" i2="3" l="ENG"><s0>Atomic force microscopy</s0>
<s5>14</s5>
</fC03>
<fC03 i1="15" i2="3" l="FRE"><s0>Cuivre</s0>
<s2>NC</s2>
<s5>15</s5>
</fC03>
<fC03 i1="15" i2="3" l="ENG"><s0>Copper</s0>
<s2>NC</s2>
<s5>15</s5>
</fC03>
<fC03 i1="16" i2="3" l="FRE"><s0>Or</s0>
<s2>NC</s2>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="3" l="ENG"><s0>Gold</s0>
<s2>NC</s2>
<s5>16</s5>
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<fC03 i1="17" i2="X" l="FRE"><s0>Oxyde d'étain</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="ENG"><s0>Tin oxide</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="SPA"><s0>Estaño óxido</s0>
<s5>17</s5>
</fC03>
<fC03 i1="18" i2="X" l="FRE"><s0>Oxyde d'indium</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="ENG"><s0>Indium oxide</s0>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="SPA"><s0>Indio óxido</s0>
<s5>18</s5>
</fC03>
<fC03 i1="19" i2="X" l="FRE"><s0>Coefficient diffusion</s0>
<s5>29</s5>
</fC03>
<fC03 i1="19" i2="X" l="ENG"><s0>Diffusion coefficient</s0>
<s5>29</s5>
</fC03>
<fC03 i1="19" i2="X" l="SPA"><s0>Coeficiente difusión</s0>
<s5>29</s5>
</fC03>
<fC03 i1="20" i2="X" l="FRE"><s0>Régime hors équilibre</s0>
<s5>30</s5>
</fC03>
<fC03 i1="20" i2="X" l="ENG"><s0>Non equilibrium conditions</s0>
<s5>30</s5>
</fC03>
<fC03 i1="20" i2="X" l="SPA"><s0>Régimen fuera equilibrio</s0>
<s5>30</s5>
</fC03>
<fC03 i1="21" i2="3" l="FRE"><s0>Longueur diffusion</s0>
<s5>31</s5>
</fC03>
<fC03 i1="21" i2="3" l="ENG"><s0>Scattering lengths</s0>
<s5>31</s5>
</fC03>
<fC03 i1="22" i2="3" l="FRE"><s0>Etude théorique</s0>
<s5>32</s5>
</fC03>
<fC03 i1="22" i2="3" l="ENG"><s0>Theoretical study</s0>
<s5>32</s5>
</fC03>
<fC03 i1="23" i2="3" l="FRE"><s0>Ni</s0>
<s4>INC</s4>
<s5>46</s5>
</fC03>
<fC03 i1="24" i2="3" l="FRE"><s0>Substrat or</s0>
<s4>INC</s4>
<s5>47</s5>
</fC03>
<fC03 i1="25" i2="3" l="FRE"><s0>Substrat InSnO</s0>
<s4>INC</s4>
<s5>48</s5>
</fC03>
<fC03 i1="26" i2="3" l="FRE"><s0>8115P</s0>
<s4>INC</s4>
<s5>71</s5>
</fC03>
<fC03 i1="27" i2="3" l="FRE"><s0>8110A</s0>
<s4>INC</s4>
<s5>72</s5>
</fC03>
<fC03 i1="28" i2="3" l="FRE"><s0>8107</s0>
<s4>INC</s4>
<s5>73</s5>
</fC03>
<fN21><s1>145</s1>
</fN21>
<fN44 i1="01"><s1>OTO</s1>
</fN44>
<fN82><s1>OTO</s1>
</fN82>
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Role of substrate in the surface diffusion and kinetic roughening of nanocrystallised nickel electrodeposits

Role of substrate in the surface diffusion and kinetic roughening of nanocrystallised nickel electrodeposits

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